【標(biāo)題速讀】【Advmat】【2022年】【1月】

2023-07-06 09:23 作者:Rt_Cola 0人讀過 | 我要投稿

聲明：本專欄主要對(duì)生命科學(xué)領(lǐng)域的一些期刊文章標(biāo)題進(jìn)行翻譯，所有內(nèi)容均由本人手工整理翻譯。由于本人專業(yè)為生物分析相關(guān)，其他領(lǐng)域如果出現(xiàn)翻譯錯(cuò)誤請(qǐng)諒解。

Anode-Free Batteries

In article number 2106005, Hui Dong, David Mitlin, and co-workers report an intermetallic for anode-free batteries. The winter scene shows a birthday cake with lit candles that are melting: the cake represents the complex structure of a cycled sodium-metal anode with the protruding candles being the dendrites. A slice, obtained by cryogenic focused ion beam (FIB) microscopy, further reveals the underlying porosity that develops during repeated plating and stripping of the metal. The thick non-uniform red frosting on the cake represents the unstable solid electrolyte interphase (SEI) that drives the dendrite growth.

無陽極電池

在文章編號(hào) 2106005 中，Hui Dong、David Mitlin 及其同事報(bào)告了一種用于無陽極電池的金屬間化合物。冬天的場(chǎng)景展示了一個(gè)生日蛋糕，上面點(diǎn)燃的蠟燭正在融化：蛋糕代表了循環(huán)鈉金屬陽極的復(fù)雜結(jié)構(gòu)，突出的蠟燭是枝晶。通過低溫聚焦離子束 (FIB) 顯微鏡獲得的切片進(jìn)一步揭示了金屬重復(fù)電鍍和剝離過程中形成的潛在孔隙度。蛋糕上厚厚的、不均勻的紅色糖霜代表了驅(qū)動(dòng)枝晶生長的不穩(wěn)定的固體電解質(zhì)界面（SEI）。

Organic Light-Emitting Diodes

Triplet exciton harvesting via triplet–triplet annihilation, is known to generate only 40% of the total radiative excitons in organic light-emitting diodes (OLEDs) theoretically. In article number 2100161, Yun-Hi Kim, Jang-Joo Kim, and co-workers realize a total radiative exciton ratio of nearly 50% with a carefully designed anthracene derivative and device structure, breaking the theoretical efficiency limit of OLEDs based on anthracene derivatives.

有機(jī)發(fā)光二極管

理論上，通過三重態(tài)-三重態(tài)湮滅收集三重態(tài)激子僅產(chǎn)生有機(jī)發(fā)光二極管 (OLED) 中總輻射激子的 40%。在第2100161號(hào)文章中，Yun-Hi Kim、Jang-Joo Kim等人通過精心設(shè)計(jì)的蒽衍生物和器件結(jié)構(gòu)實(shí)現(xiàn)了近50%的總輻射激子比，突破了基于蒽衍生物的OLED的理論效率極限。

Deep-UV Photodetectors

High-performance harsh-environment-resistant deep-UV (DUV) photodetectors have important applications in space exploration and flame prewarning. In article number 2106923, Xiaolong Zhao, Shibing Long, and co-workers tailor defect/doping engineering based on the low-cost GaOX to obtain high-performance DUV detectors. The defect/doping engineering induces recrystallization, doping compensation, and nanopore formation inside the material, giving it great potential for DUV detection in harsh conditions.

深紫外光電探測(cè)器

高性能耐惡劣環(huán)境的深紫外（DUV）光電探測(cè)器在太空探索和火焰預(yù)警方面具有重要應(yīng)用。在第 2106923 號(hào)文章中，Xiaolong Zhao、Shibing Long 及其同事基于低成本 GaOX 定制了缺陷/摻雜工程，以獲得高性能 DUV 探測(cè)器。缺陷/摻雜工程引起材料內(nèi)部的再結(jié)晶、摻雜補(bǔ)償和納米孔的形成，使其在惡劣條件下的 DUV 檢測(cè)具有巨大的潛力。

Bioprinting

In article number 2107038, Yu Shrike Zhang and co-workers develop a (bio)printing system based on Digital Light Processing to utilize the integration of a microfluidic mixer for the generation of either continual or discrete gradients of desired (bio)inks in real time. As such, the precisely controlled gradients are composable on-the-fly by facilely adjusting the (bio)ink flow ratios, supporting the potential of the platform in numerous biomedical applications.

生物打印

在文章編號(hào) 2107038 中，Yu Shrike Zhang 和同事開發(fā)了一種基于數(shù)字光處理的（生物）打印系統(tǒng)，利用微流體混合器的集成實(shí)時(shí)生成所需（生物）墨水的連續(xù)或離散梯度。因此，通過輕松調(diào)整（生物）墨水流量比率，可以即時(shí)組合精確控制的梯度，從而支持該平臺(tái)在眾多生物醫(yī)學(xué)應(yīng)用中的潛力。

Strain Engineering

In article number 2103571, Roberto D'Agosta, Andres Castellanos-Gomez, and co-workers report a method to apply uniaxial strain along different crystal orientations and apply the method to study the strain-tunability of excitons in zirconium triselenide, a 2D semiconductor with an interesting in-plane anisotropic crystal structure.

應(yīng)變工程

在文章編號(hào) 2103571 中，Roberto D'Agosta、Andres Castellanos-Gomez 及其同事報(bào)告了一種沿不同晶體取向施加單軸應(yīng)變的方法，并應(yīng)用該方法研究三硒化鋯（一種二維半導(dǎo)體）中激子的應(yīng)變可調(diào)性。有趣的面內(nèi)各向異性晶體結(jié)構(gòu)。

Artificial Biomolecular Condensates

In article number 2104704, Huaimin Wang and co-workers report a general approach for constructing artificial biomolecular condensates of oligopeptide in living cells. The rationally designed aromatic-capped peptides can reversibly form a nanofibrous hydrogel with a change of the conformation and morphologies in the lysosome. The formed condensates undergo swelling in the lysosome, leading to lysosomal membrane permeabilization and re-direction of therapeutic drugs to the target.

人造生物分子凝聚體

在第 2104704 號(hào)文章中，王懷民及其同事報(bào)告了一種在活細(xì)胞中構(gòu)建寡肽人工生物分子縮合物的一般方法。合理設(shè)計(jì)的芳香肽可以在溶酶體中可逆地形成納米纖維水凝膠，并改變其構(gòu)象和形態(tài)。形成的冷凝物在溶酶體中膨脹，導(dǎo)致溶酶體膜透化并將治療藥物重定向至靶點(diǎn)。

Tadf Emitters

Circularly polarized thermally activated delayed fluorescence (CP-TADF) and multiple-resonance thermally activated delayed fluorescence (MR-TADF) properties are integrated into new CPMR-TADF materials by Xiugang Wu, You-Xuan Zheng, Weiguo Zhu, Pi-Tai Chou, and co-workers, as described in article number 2105080. Organic light-emitting diodes based on these CPMR-TADF emitters attain a three-in-one advantage simultaneously: high efficiency, color purity, and circular polarized light.

塔德夫發(fā)射器

Xiugang Wu、You-Xuan Cheng、Weiguo Zhu、Pi-Tai Chou 將圓偏振熱激活延遲熒光 (CP-TADF) 和多重共振熱激活延遲熒光 (MR-TADF) 特性集成到新型 CPMR-TADF 材料中和同事，如文章編號(hào) 2105080 中所述?；谶@些 CPMR-TADF 發(fā)射器的有機(jī)發(fā)光二極管同時(shí)具有三合一優(yōu)勢(shì)：高效率、色純度和圓偏振光。

Electro-Actuation

In article number 2105923, Manuel Brinker and Patrick Huber report laser cantilever bending experiments that show large and reversible electrosorption-induced deformation of wafer-scale nanoporous silicon in aqueous electrolytes (isotonic saline solution) at exceptionally small operation voltages. This paves the way for on-chip integrated actuation and stress generation, e.g., in (bio-)medical environments, as is illustrated by electro-mechanical stimulation of living cells.

電驅(qū)動(dòng)

在文章編號(hào) 2105923 中，Manuel Brinker 和 Patrick Huber 報(bào)告了激光懸臂彎曲實(shí)驗(yàn)，該實(shí)驗(yàn)表明，在極小的工作電壓下，在水性電解質(zhì)（等滲鹽水溶液）中，晶圓級(jí)納米多孔硅會(huì)發(fā)生大且可逆的電吸附引起的變形。這為片上集成驅(qū)動(dòng)和應(yīng)力生成鋪平了道路，例如在（生物）醫(yī)學(xué)環(huán)境中，如活細(xì)胞的機(jī)電刺激所示。

Tumor Therapy

In article number 2106606, Nan Qin, Tiger H. Tao, and co-workers report a heterogenous silk microneedle patch to spatiotemporally and sequentially deliver multiple therapeutic drugs for hemostasis, anti-angiogenesis, and apoptosis of brain tumor cells. Drug release kinetics are well-defined by tuning the crosslinking degree of the silk and applying a trigger of transcranial NIR-light irradiation. This biodegradable patch has potential applications for the clinical treatment of intracranial tumors.

腫瘤治療

在第 2106606 號(hào)文章中，Nanqin、TigerH.Tao 及其同事報(bào)道了一種異質(zhì)絲微針貼片，可在時(shí)空上順序輸送多種治療藥物，用于止血、抗血管生成和腦腫瘤細(xì)胞凋亡。通過調(diào)節(jié)絲的交聯(lián)度并應(yīng)用經(jīng)顱近紅外光照射的觸發(fā)，可以明確藥物釋放動(dòng)力學(xué)。這種可生物降解的貼片在顱內(nèi)腫瘤的臨床治療方面具有潛在的應(yīng)用前景。

Perovskite Solar Cells

Light-intensity analysis of JV parameters is introduced by Yulia Galagan and Damian Glowienka in article number 2105920 as a simple method to allow understanding of the dominating mechanisms that limit device performance in perovskite solar cells. The method is based on the drift–diffusion model and is aimed at helping in the explanation of parasitic losses from trap-assisted recombination or ohmic losses in devices.

鈣鈦礦太陽能電池

Yulia Galagan 和 Damian Glowienka 在文章編號(hào) 2105920 中介紹了 JV 參數(shù)的光強(qiáng)度分析，這是一種簡(jiǎn)單的方法，可以幫助了解限制鈣鈦礦太陽能電池器件性能的主要機(jī)制。該方法基于漂移擴(kuò)散模型，旨在幫助解釋來自陷阱輔助復(fù)合的寄生損耗或器件中的歐姆損耗。

Personalized Antibiotherapy

In article number 2104555, Can Dincer and co-workers introduce an electrochemical multiplexed biosensor combined with a synthetic-biology-empowered assay, which enables a simple, yet accurate method to provide insights regarding the antibiotic levels even in exhaled breath condensate. The validated findings demonstrate the potential of the system to shift the paradigm of the “one size-fits-all” strategy for combating antibiotic resistance.

個(gè)性化抗生素治療

在文章編號(hào) 2104555 中，Can Dincer 及其同事介紹了一種電化學(xué)多重生物傳感器與合成生物學(xué)授權(quán)檢測(cè)相結(jié)合，該方法提供了一種簡(jiǎn)單而準(zhǔn)確的方法，即使在呼出的呼吸冷凝液中也能提供有關(guān)抗生素水平的見解。經(jīng)驗(yàn)證的結(jié)果表明，該系統(tǒng)有潛力改變對(duì)抗抗生素耐藥性的“一刀切”策略范式。

Embolization

In article number 2106865, Fiorenzo Omenetto, Rahmi Oklu, and co-workers demonstrate a silk embolic material (represented in yellow) being released from a catheter and occluding an artery. Therapeutics within the silk embolic material (shown in blue) diffusing outside of the arterial wall achieve targeted drug delivery within the tissue parenchyma.

栓塞術(shù)

在第 2106865 號(hào)文章中，F(xiàn)iorenzo Omenetto、Rahmi Oklu 及其同事演示了絲栓塞材料（以黃色表示）從導(dǎo)管中釋放并閉塞動(dòng)脈。絲栓塞材料（以藍(lán)色顯示）內(nèi)的治療藥物擴(kuò)散到動(dòng)脈壁外，實(shí)現(xiàn)組織實(shí)質(zhì)內(nèi)的靶向藥物輸送。

Nanocrystal Dislocations

Inducing dislocations is an efficient approach to generate strain effects in nanomaterials. In article number 2106973, Yanan Chen and co-workers report a non-equilibrium high-temperature thermal-shock method (HTS) to induce dislocations in nanocrystals by using liquid nitrogen. The dislocations induced by thermal and structural stress are frozen in nanoparticles. The extreme environmental HTS can introduce dislocations in Pt nanoparticles and improve hydrogen evolution reaction performance.

納米晶體位錯(cuò)

誘導(dǎo)位錯(cuò)是在納米材料中產(chǎn)生應(yīng)變效應(yīng)的有效方法。在文章編號(hào) 2106973 中，Yanan Chen 及其同事報(bào)告了一種使用液氮誘導(dǎo)納米晶體位錯(cuò)的非平衡高溫?zé)釠_擊方法 (HTS)。由熱應(yīng)力和結(jié)構(gòu)應(yīng)力引起的位錯(cuò)被凍結(jié)在納米顆粒中。極端環(huán)境高溫超導(dǎo)可以在Pt納米粒子中引入位錯(cuò)并提高析氫反應(yīng)性能。

Cancer Therapy

In article number 2100096, Olivier Elemento, Ankur Singh, and co-workers examine the prostate cancer tumor microenvironment using multi-omics techniques and report a prostate cancer organoid bioengineered using a modular synthetic hydrogel that shapes the epigenetics and transcriptomics of cancer cells. They discover the “dopamine receptor” pathway as a targeted therapy for epigenetically reprogrammed neuroendocrine prostate cancers.

癌癥治療

在第 2100096 號(hào)文章中，Olivier Elemento、Ankur Singh 及其同事使用多組學(xué)技術(shù)檢查了前列腺癌腫瘤微環(huán)境，并報(bào)告了使用模塊化合成水凝膠進(jìn)行生物工程改造的前列腺癌類器官，該水凝膠塑造了癌細(xì)胞的表觀遺傳學(xué)和轉(zhuǎn)錄組學(xué)。他們發(fā)現(xiàn)“多巴胺受體”途徑可作為表觀遺傳重編程神經(jīng)內(nèi)分泌前列腺癌的靶向治療。

Lithium–Sulfur Batteries

A “Quasi-MOF” nanosphere is introduced by Yongguang Zhang, Xin Wang, Zhongwei Chen, and co-workers in article number 2105541 as an efficient and durable sulfur electrocatalyst toward accelerated sulfur reduction reaction. The reversible de-ligandation/ligandation of this Quasi-MOF over the course of the electrochemical process endows its with excellent catalytic activity and remarkable durability. Attributed to these structural advantages, the Quasi-MOF delivers a decent discharge capacity and low-capacity fading rate over long-term cycling.

鋰硫電池

Yongguang Zhang、Xin Wang、Zhongwei Chen 及其同事在文章編號(hào) 2105541 中介紹了一種“準(zhǔn) MOF”納米球，作為一種高效且耐用的硫電催化劑，可加速硫還原反應(yīng)。這種準(zhǔn)MOF在電化學(xué)過程中可逆的脫配位/配位賦予其優(yōu)異的催化活性和卓越的耐久性。由于這些結(jié)構(gòu)優(yōu)勢(shì)，準(zhǔn) MOF 在長期循環(huán)中具有良好的放電容量和低容量衰減率。

Broad-Spectrum Photodetection

In article number 2107206, Yue-Yang Liu, Zhongming Wei, and co-workers show how upward movement of the Fermi level enables multichannel transition of electrons. This mechanism achieves a broad spectral response in a PdPS-based photodetector. In addition, the PdPS-based polarization-sensitive photodetector and polarimetric image sensor realize the application of object detection.

廣譜光電檢測(cè)

在第 2107206 號(hào)文章中，Yue-Yang Liu、Zhongming Wei 及其同事展示了費(fèi)米能級(jí)的向上運(yùn)動(dòng)如何實(shí)現(xiàn)電子的多通道躍遷。這種機(jī)制在基于 PdPS 的光電探測(cè)器中實(shí)現(xiàn)了寬光譜響應(yīng)。此外，基于PdPS的偏振敏感光電探測(cè)器和偏振圖像傳感器實(shí)現(xiàn)了物體檢測(cè)的應(yīng)用。

Nanomechanical Resonators

In article number 2106248, Miguel A. Bessa, Richard A. Norte, and co-workers report the design of a nature-inspired spiderweb sensor using artificial intelligence and discover a novel vibration mechanism. The device's world-class performance is verified experimentally, opening avenues toward ultrasensitive detection of fundamental forces and quantum technologies operating at room temperature.

納米機(jī)械諧振器

在第 2106248 號(hào)文章中，Miguel A. Bessa、Richard A. Norte 及其同事報(bào)告了利用人工智能設(shè)計(jì)的受自然啟發(fā)的蜘蛛網(wǎng)傳感器，并發(fā)現(xiàn)了一種新穎的振動(dòng)機(jī)制。該設(shè)備的世界級(jí)性能經(jīng)過實(shí)驗(yàn)驗(yàn)證，為超靈敏檢測(cè)基本力和在室溫下運(yùn)行的量子技術(shù)開辟了途徑。

Liquid Gating

Liquid-gating technology is attracting increasing attention for the delivery of some brand-new properties for real-world applications. In article number 2107327, Xu Hou and co-workers report a self-driven smart liquid-gating system, developed by designing a liquid-gating magnetoelastic porous membrane with reversible meniscus-shaped deformations. This system provides a universal and convenient way to realize active regulation of gas/liquid release. The illustrated visible gas/liquid-mixture content monitoring showcases one example of the application of the reported material.

液體澆口

液體澆注技術(shù)因?yàn)閷?shí)際應(yīng)用提供一些全新特性而受到越來越多的關(guān)注。在第2107327號(hào)文章中，Xu Hou和同事報(bào)告了一種自驅(qū)動(dòng)智能液體澆注系統(tǒng)，該系統(tǒng)通過設(shè)計(jì)具有可逆彎月形變形的液體澆注磁致彈性多孔膜而開發(fā)。該系統(tǒng)為實(shí)現(xiàn)氣/液釋放的主動(dòng)調(diào)節(jié)提供了一種通用且便捷的方法。圖示的可見氣體/液體混合物含量監(jiān)測(cè)展示了所報(bào)告材料的應(yīng)用的一個(gè)示例。

Wound Healing

In article number 2106842, Miaomiao Yuan, Daxiang Cui, Hossam Haick, and co-workers report a novel self-healing elastomer-based multifunctional wound dressing (MFWD) with desirable mechanical robustness, biocompatibility, and antibacterial activity for effective wound management. MFWD assists in contracting wound edges, based on the excellent self-healing ability of the elastomer, and enables tracking of the wound health status in real-time via a set of (bio)chemical and physical sensors integrated therein.

傷口愈合

在第 2106842 號(hào)文章中，Miaomiao Yuan、Dayang Cui、Hossam Haick 及其同事報(bào)告了一種新型自修復(fù)彈性體多功能傷口敷料 (MFWD)，其具有理想的機(jī)械堅(jiān)固性、生物相容性和抗菌活性，可用于有效的傷口管理。 MFWD 基于彈性體優(yōu)異的自愈能力，有助于收縮傷口邊緣，并通過其中集成的一組（生物）化學(xué)和物理傳感器實(shí)時(shí)跟蹤傷口健康狀態(tài)。

Lithium-Ion Batteries

In article number 2106402, Mark C. Hersam and co-workers show that lattice oxygen loss plays a critical role in the O3–O1 stacking transition in cobalt-free LiNiO2 lithium-ion battery cathodes, which subsequently induces Ni-ion migration and irreversible stacking faults, microscale electrochemical creep, cracking, and even bending of layers after high-voltage cycling. By suppressing oxygen evolution, hermetic graphene coatings arrest this degradation cascade, resulting in substantially improved high-voltage capacity retention.

鋰離子電池

在文章編號(hào) 2106402 中，Mark C. Hersam 及其同事表明，晶格氧損失在無鈷 LiNiO2 鋰離子電池陰極的 O3-O1 堆積轉(zhuǎn)變中起著關(guān)鍵作用，隨后誘導(dǎo) Ni 離子遷移和不可逆堆積高壓循環(huán)后層的缺陷、微觀電化學(xué)蠕變、開裂甚至彎曲。通過抑制析氧，密封石墨烯涂層可以阻止這種級(jí)聯(lián)降解，從而顯著提高高壓容量保持率。

Near-Surface Doping

In article number 2103235, David N. Jamieson and co-workers report that single-crystal silicon can be configured with arrays of single, near-surface, dopant atoms using on-chip electrodes and low-noise charge-sensitive electronics to register single-ion implants. Suitable for integration with a nanostencil scanner to localize the implants, the system makes use of the signal of electron–hole pairs generated as the ions dissipate their kinetic energy in the crystal. The system can be part of an engineering strategy for high-confidence fabrication of large-scale donor arrays to exploit donor spin ensembles in silicon devices.

近表面摻雜

在文章編號(hào) 2103235 中，David N. Jamieson 和同事報(bào)告單晶硅可以配置有單個(gè)近表面摻雜原子陣列，使用片上電極和低噪聲電荷敏感電子器件來記錄單離子注入。該系統(tǒng)適合與納米模板掃描儀集成以定位植入物，利用離子在晶體中耗散動(dòng)能時(shí)產(chǎn)生的電子空穴對(duì)信號(hào)。該系統(tǒng)可以成為高可信度制造大規(guī)模施主陣列的工程策略的一部分，以利用硅器件中的施主自旋系綜。

Molecular Sieves

In article number 2105156, Tai-Shung Chung and co-workers show how soluble organic macrocyclic cavitands (OMCs) with interactive affinity for polymers can be utilized to design novel nanocomposite membranes with true molecular homogeneity, unlike conventional nanoarchitectures that form heterogeneous nanofiller phases within membranes that cause performance and processability issues. By adjusting the OMC cavity size within the membranes, tunable gas-transport properties can be obtained for molecular-sieving H2/CO2 separation.

分子篩

在文章編號(hào) 2105156 中，Tai-Shung Chung 及其同事展示了如何利用對(duì)聚合物具有交互親和力的可溶性有機(jī)大環(huán)空配體 (OMC) 來設(shè)計(jì)具有真正分子均質(zhì)性的新型納米復(fù)合膜，這與在膜內(nèi)形成異質(zhì)納米填料相的傳統(tǒng)納米結(jié)構(gòu)不同導(dǎo)致性能和可加工性問題。通過調(diào)節(jié)膜內(nèi)的 OMC 空腔尺寸，可以獲得可調(diào)節(jié)的氣體傳輸特性，用于分子篩 H2/CO2 分離。

2D Materials

In article number 2106674, Kai Xiao and co-workers develop a nonequilibrium chemical vapor deposition approach for selective formation of antisite defects in atomically thin 2D tungsten sulfide monolayer crystals by regulating the diffusion of tungsten into gold substrates. This work demonstrates a novel strategy for the selective formation of defects in 2D materials by tuning their formation energy during synthesis via choice of substrate and alloy design.

二維材料

在文章編號(hào) 2106674 中，Kaiiao 及其同事開發(fā)了一種非平衡化學(xué)氣相沉積方法，通過調(diào)節(jié)鎢向金基底的擴(kuò)散，在原子薄的二維硫化鎢單層晶體中選擇性形成反位缺陷。這項(xiàng)工作展示了一種在二維材料中選擇性形成缺陷的新策略，通過選擇基材和合金設(shè)計(jì)來調(diào)整合成過程中的形成能。

Programmable Liquid Droplets

In article number 2104837, Umberto Capasso Palmiero, Paolo Arosio, and co-workers propose a strategy to produce programmable liquid droplets via liquid–liquid phase separation of associative zwitterionic polymers. With this approach, multiple properties of the droplets, such as composition and stimulus responsiveness, can be finely tuned, opening attractive applications in bioseparation and diagnostics.

可編程液滴

在第 2104837 號(hào)文章中，Umberto Capasso Palmiero、Paolo Arosio 及其同事提出了一種通過締合兩性離子聚合物的液-液相分離來生產(chǎn)可編程液滴的策略。通過這種方法，可以微調(diào)液滴的多種特性，例如成分和刺激響應(yīng)性，從而在生物分離和診斷中開辟有吸引力的應(yīng)用。

Stretchable Phototransistors

In article number 2107304, Yunlong Guo and co-workers achieve intrinsically stretchable phototransistors based on a designed polymer/perovskite heterojunction. The obtained stretchable phototransistors show a high-sensitivity response to high-energy photons (e.g. X-rays or UV light) even under 100% tensile strain. Some other optoelectronic skin characteristics, high sensing specificity, high transmittance, high tolerance to harsh mechanical deformations, and superior skin conformability, are also demonstrated.

可拉伸光電晶體管

在第 2107304 號(hào)文章中，郭云龍和同事基于設(shè)計(jì)的聚合物/鈣鈦礦異質(zhì)結(jié)實(shí)現(xiàn)了本質(zhì)上可拉伸的光電晶體管。所獲得的可拉伸光電晶體管即使在 100% 拉伸應(yīng)變下也表現(xiàn)出對(duì)高能光子（例如 X 射線或紫外線）的高靈敏度響應(yīng)。還展示了其他一些光電皮膚特性，例如高傳感特異性、高透射率、對(duì)嚴(yán)酷機(jī)械變形的高耐受性以及卓越的皮膚順應(yīng)性。

Additive-Free Inks

Additive-free dry-only inks can enable functional printing and high-throughput fabrication of elec-tronics at room temperature, but their design proves challenging. In article number 2103660, Jakob Heier and co-workers show how interflake van der Waals interactions in 2D materials can be used to replace the roles of conventional additives for the formulation of additive-free inks.

無添加劑墨水

無添加劑的干油墨可以在室溫下實(shí)現(xiàn)功能性印刷和電子產(chǎn)品的高通量制造，但其設(shè)計(jì)被證明具有挑戰(zhàn)性。在文章編號(hào) 2103660 中，Jakob Heier 及其同事展示了如何利用二維材料中的片間范德華相互作用來替代傳統(tǒng)添加劑的作用，以配制無添加劑油墨。

Quantum-Dot Light-Emitting Diodes

Light-emitting diodes (LEDs) in a tandem configuration offer a strategy to realize high-performance, multi-color devices, but the efficiency of tandem quantum-dot based LEDs (QLEDs) has been limited due to unpassivated interfaces and solvent damage originating from the materials processing requirements of the interconnecting layers (ICLs). In article number 2108150, Edward H. Sargent, Xuyong Yang, and co-workers report an ICL consisting of a semiconductor–metal–dielectric stack that provides facile fabrication, materials stability, and good optoelectronic coupling, making the tandem QLED based on the ICL achieve recording efficiency.

量子點(diǎn)發(fā)光二極管

串聯(lián)配置的發(fā)光二極管（LED）提供了一種實(shí)現(xiàn)高性能多色器件的策略，但由于互連層（ICL）的材料加工要求導(dǎo)致的未鈍化界面和溶劑損壞，串聯(lián)量子點(diǎn)基LED（QLED）的效率受到限制。在文章編號(hào)2108150中，Edward H.Sargent、Xuyong Yang及其同事報(bào)道了一種由半導(dǎo)體-金屬-電介質(zhì)堆疊組成的ICL，該堆疊提供了易于制造、材料穩(wěn)定性和良好的光電耦合，使基于ICL的串聯(lián)QLED實(shí)現(xiàn)了記錄效率。

3D Printing

In article number 2107249, Lei Wu, Yanlin Song, and co-workers propose a continuous liquid film confined 3D printing strategy to fabricate high-precision 3D structures. Reutilization and good control of the liquid residual can improve the printing fidelity and avoid a post-washing process. A centimeter-scale contact-lens structure with nanoscale roughness, high-definition imaging and homogeneous mechanical characteristic is printed, indicating its great potential in scalable 3D printing of optical structures.

3D打印

在第 2107249 號(hào)文章中，Lei Wu、Yanlin Song 及其同事提出了一種連續(xù)液膜限制 3D 打印策略來制造高精度 3D 結(jié)構(gòu)。液體殘留的再利用和良好控制可以提高印刷保真度并避免后清洗過程。打印出具有納米級(jí)粗糙度、高清成像和均勻機(jī)械特性的厘米級(jí)隱形眼鏡結(jié)構(gòu)，表明其在可擴(kuò)展的光學(xué)結(jié)構(gòu)3D打印方面具有巨大潛力。

Photonic Pigments

In article number 2107398, Yadong Yin and co-workers highlight the integration of magnetically responsive photonic pigments with orientation-dependent structural colors into optoelectronic devices that can exhibit dynamic color-switching or display predesigned patterns upon simple rotation. Such photonic pigments are promising materials in the development of high-performance sensors, color displays, rewritable papers, and anti-counterfeiting devices.

光子顏料

在第 2107398 號(hào)文章中，Yadong Yin 及其同事重點(diǎn)介紹了將具有方向相關(guān)結(jié)構(gòu)顏色的磁響應(yīng)光子顏料集成到光電器件中，這些器件可以在簡(jiǎn)單旋轉(zhuǎn)時(shí)表現(xiàn)出動(dòng)態(tài)顏色切換或顯示預(yù)先設(shè)計(jì)的圖案。這種光子顏料是開發(fā)高性能傳感器、彩色顯示器、可重寫紙和防偽設(shè)備的有前途的材料。

Fluorescent Patterning

In article number 2107452, Wei Lu, Tao Chen, and co-workers present a photomechanically modulated fluorescent system that enables on-demand display of fluorescent patterns under near-IR light light via photomechanical bending of a fluorescent actuator. This strategy is promising for fabricating on-demand fluorescent display platforms that combine a wide choice of fluorophores, remote control with high spatial/temporal precision, and single-input multiple-output features.

熒光圖案

在文章編號(hào) 2107452 中，Wei Lu、Tao Chen 及其同事提出了一種光機(jī)械調(diào)制熒光系統(tǒng)，該系統(tǒng)能夠通過熒光致動(dòng)器的光機(jī)械彎曲在近紅外光下按需顯示熒光圖案。該策略有望用于制造按需熒光顯示平臺(tái)，該平臺(tái)結(jié)合了多種熒光團(tuán)選擇、具有高空間/時(shí)間精度的遠(yuǎn)程控制以及單輸入多輸出功能。

1.Understanding the Role of Lithium Iodide in Lithium–Oxygen Batteries.

了解碘化鋰在鋰氧電池中的作用。

2.Fiber-Based Biopolymer Processing as a Route toward Sustainability.

基于纖維的生物聚合物加工作為可持續(xù)發(fā)展的途徑。

3.Tin Halide Perovskites: From Fundamental Properties to Solar Cells.

鹵化錫鈣鈦礦：從基本特性到太陽能電池。

4.Recent Advances in Fluorinated Graphene from Synthesis to Applications: Critical Review on Functional Chemistry and Structure Engineering.

氟化石墨烯從合成到應(yīng)用的最新進(jìn)展：功能化學(xué)和結(jié)構(gòu)工程的批判性評(píng)論。

5.Bimetallic Janus Nanocrystals: Syntheses and Applications.

雙金屬 Janus 納米晶體：合成和應(yīng)用。

6.Machine Learning-Driven Biomaterials Evolution.

機(jī)器學(xué)習(xí)驅(qū)動(dòng)的生物材料進(jìn)化。

7.Advanced Point-of-Care Testing Technologies for Human Acute Respiratory Virus Detection.

用于人類急性呼吸道病毒檢測(cè)的先進(jìn)護(hù)理點(diǎn)檢測(cè)技術(shù)。

8.Bioinspired and Biomimetic Delivery Platforms for Cancer Vaccines.

癌癥疫苗的仿生和仿生遞送平臺(tái)。

9.Processing of Self-Healing Polymers for Soft Robotics.

用于軟機(jī)器人的自修復(fù)聚合物的加工。

10.A Sodium–Antimony–Telluride Intermetallic Allows Sodium-Metal Cycling at 100% Depth of Discharge and as an Anode-Free Metal Battery.

鈉-銻-碲化物金屬間化合物允許鈉-金屬在 100% 放電深度下循環(huán)，并可作為無陽極金屬電池。

11.Breaking the Efficiency Limit of Deep-Blue Fluorescent OLEDs Based on Anthracene Derivatives.

突破基于蒽衍生物的深藍(lán)色熒光 OLED 的效率極限。

12.High-Performance Harsh-Environment-Resistant GaOX Solar-Blind Photodetectors via Defect and Doping Engineering.

通過缺陷和摻雜工程實(shí)現(xiàn)高性能耐惡劣環(huán)境的 GaOX 日盲光電探測(cè)器。

13.Digital Light Processing Based Bioprinting with Composable Gradients.

基于數(shù)字光處理的具有可組合梯度的生物打印。

14.Strongly Anisotropic Strain-Tunability of Excitons in Exfoliated ZrSe3.

剝離 ZrSe3 中激子的強(qiáng)各向異性應(yīng)變可調(diào)性。

15.Intracellular Condensates of Oligopeptide for Targeting Lysosome and Addressing Multiple Drug Resistance of Cancer.

用于靶向溶酶體并解決癌癥多重耐藥性的寡肽細(xì)胞內(nèi)縮合物。

16.Fabrication of Circularly Polarized MR-TADF Emitters with Asymmetrical Peripheral-Lock Enhancing Helical B/N-Doped Nanographenes.

使用不對(duì)稱外圍鎖增強(qiáng)螺旋 B/N 摻雜納米石墨烯制造圓偏振 MR-TADF 發(fā)射器。

17.Wafer-Scale Electroactive Nanoporous Silicon: Large and Fully Reversible Electrochemo-Mechanical Actuation in Aqueous Electrolytes.

晶圓級(jí)電活性納米多孔硅：水電解質(zhì)中的大型且完全可逆的電化學(xué)機(jī)械驅(qū)動(dòng)。

18.Silk Microneedle Patch Capable of On-Demand Multidrug Delivery to the Brain for Glioblastoma Treatment.

絲質(zhì)微針貼片能夠按需向大腦輸送多種藥物以治療膠質(zhì)母細(xì)胞瘤。

19.Manipulating Color Emission in 2D Hybrid Perovskites by Fine Tuning Halide Segregation: A Transparent Green Emitter.

通過微調(diào)鹵化物偏析來控制二維混合鈣鈦礦中的顏色發(fā)射：透明的綠色發(fā)射體。

20.Cycloruthenated Self-Assembly with Metabolic Inhibition to Efficiently Overcome Multidrug Resistance in Cancers.

環(huán)釕自組裝具有代謝抑制作用，可有效克服癌癥的多藥耐藥性。

21.Strain-Enabled Phase Transition of Periodic Metasurfaces.

周期性超表面的應(yīng)變啟用相變。

22.Conjugated Polymer Mesocrystals with Structural and Optoelectronic Coherence and Anisotropy in Three Dimensions.

具有結(jié)構(gòu)和光電相干性以及三維各向異性的共軛聚合物介晶。

23.Designing a Zn–Ag Catalyst Matrix and Electrolyzer System for CO2 Conversion to CO and Beyond.

設(shè)計(jì)用于將 CO2 轉(zhuǎn)化為 CO 及其他物質(zhì)的 Zn-Ag 催化劑基質(zhì)和電解槽系統(tǒng)。

24.Controllable SiOx Nanorod Memristive Neuron for Probabilistic Bayesian Inference.

用于概率貝葉斯推理的可控 SiOx 納米棒憶阻神經(jīng)元。

25.Self-Complementary Zwitterionic Peptides Direct Nanoparticle Assembly and Enable Enzymatic Selection of Endocytic Pathways.

自互補(bǔ)兩性離子肽直接納米顆粒組裝并實(shí)現(xiàn)內(nèi)吞途徑的酶促選擇。

26.Investigation of the Effect of 3D Meniscus Geometry on Fluid Dynamics and Crystallization via In Situ Optical Microscopy-Assisted Mathematical Modeling.

通過原位光學(xué)顯微鏡輔助數(shù)學(xué)建模研究 3D 彎月面幾何形狀對(duì)流體動(dòng)力學(xué)和結(jié)晶的影響。

27.Loading Single-Ni Atoms on Assembled Hollow N-Rich Carbon Plates for Efficient CO2 Electroreduction.

在組裝的空心富氮碳板上負(fù)載單鎳原子以實(shí)現(xiàn)高效的 CO2 電還原。

28.Lead-Dominated Hyperfine Interaction Impacting the Carrier Spin Dynamics in Halide Perovskites.

以鉛為主的超精細(xì)相互作用影響鹵化物鈣鈦礦中的載流子自旋動(dòng)力學(xué)。

29.Enzyme Therapeutic for Ischemia and Reperfusion Injury in Organ Transplantation.

器官移植中缺血和再灌注損傷的酶治療。

30.Self-Catalytic Small Interfering RNA Nanocarriers for Synergistic Treatment of Neurodegenerative Diseases.

用于協(xié)同治療神經(jīng)退行性疾病的自催化小干擾 RNA 納米載體。

31.Liquid-Metal-Enabled Mechanical-Energy-Induced CO2 Conversion.

液態(tài)金屬機(jī)械能誘導(dǎo)二氧化碳轉(zhuǎn)化。

32.Transfer-Enabled Fabrication of Graphene Wrinkle Arrays for Epitaxial Growth of AlN Films.

用于 AlN 薄膜外延生長的石墨烯皺紋陣列的轉(zhuǎn)移制造。

33.Exploring the Pb1?xSrxHfO3 System and Potential for High Capacitive Energy Storage Density and Efficiency.

探索 Pb1?xSrxHfO3 系統(tǒng)以及高電容儲(chǔ)能密度和效率的潛力。

34.Coupling Spin Defects in a Layered Material to Nanoscale Plasmonic Cavities.

將層狀材料中的自旋缺陷與納米級(jí)等離子體腔耦合。

35.Viologen-Immobilized 2D Polymer Film Enabling Highly Efficient Electrochromic Device for Solar-Powered Smart Window.

紫精固定的二維聚合物薄膜可實(shí)現(xiàn)太陽能智能窗的高效電致變色器件。

36.Synthesis of Pd3Sn and PdCuSn Nanorods with L12 Phase for Highly Efficient Electrocatalytic Ethanol Oxidation.

合成具有 L12 相的 Pd3Sn 和 PdCuSn 納米棒，用于高效電催化乙醇氧化。

37.Mesenchymal Stem Cell-Derived Extracellular Vesicles with High PD-L1 Expression for Autoimmune Diseases Treatment.

具有高 PD-L1 表達(dá)的間充質(zhì)干細(xì)胞衍生的細(xì)胞外囊泡，用于治療自身免疫性疾病。

38.Universal Existence of Localized Single-Photon Emitters in the Perovskite Film of All-Inorganic CsPbBr3 Microcrystals.

全無機(jī) CsPbBr3 微晶鈣鈦礦薄膜中局域單光子發(fā)射體的普遍存在。

39.Spatiotemporally Controllable Distribution of Combination Therapeutics in Solid Tumors by Dually Modified Bacteria.

雙修飾細(xì)菌聯(lián)合治療在實(shí)體瘤中的時(shí)空可控分布。

40.Textured Electrodes: Manipulating Built-In Crystallographic Heterogeneity of Metal Electrodes via Severe Plastic Deformation.

紋理電極：通過嚴(yán)重塑性變形操縱金屬電極的內(nèi)置晶體異質(zhì)性。

41.Encapsulation of Metallic Zn in a Hybrid MXene/Graphene Aerogel as a Stable Zn Anode for Foldable Zn-Ion Batteries.

將金屬鋅封裝在混合 MXene/石墨烯氣凝膠中作為可折疊鋅離子電池的穩(wěn)定鋅陽極。

42.Over 21% Efficiency Stable 2D Perovskite Solar Cells.

效率超過 21% 的穩(wěn)定二維鈣鈦礦太陽能電池。

43.A High-Performance, Sensitive, Wearable Multifunctional Sensor Based on Rubber/CNT for Human Motion and Skin Temperature Detection.

一種基于橡膠/碳納米管的高性能、靈敏、可穿戴多功能傳感器，用于人體運(yùn)動(dòng)和皮膚溫度檢測(cè)。

44.Ratiometric FRET Encoded Hierarchical ZrMOF?@?Au Cluster for Ultrasensitive Quantifying MicroRNA In Vivo.

比率 FRET 編碼分層 ZrMOF @ Au 簇，用于體內(nèi)超靈敏定量 MicroRNA。

45.A Comparison of Charge Carrier Dynamics in Organic and Perovskite Solar Cells.

有機(jī)太陽能電池和鈣鈦礦太陽能電池中電荷載流子動(dòng)力學(xué)的比較。

46.Bioactive Synthetic Polymers.

生物活性合成聚合物。

47.Challenges and Strategies of Low-Cost Aluminum Anodes for High-Performance Al-Based Batteries.

高性能鋁基電池低成本鋁陽極的挑戰(zhàn)和策略。

48.3D Bioprinting of Cell-Laden Hydrogels for Improved Biological Functionality.

載有細(xì)胞的水凝膠的 3D 生物打印可改善生物功能。

49.A Critical Outlook for the Pursuit of Lower Contact Resistance in Organic Transistors.

追求有機(jī)晶體管更低接觸電阻的重要展望。

50.Emerging Electrocatalysts for Water Oxidation under Near-Neutral CO2 Reduction Conditions.

近中性二氧化碳還原條件下水氧化的新興電催化劑。

51.Light Intensity Analysis of Photovoltaic Parameters for Perovskite Solar Cells.

鈣鈦礦太陽能電池光伏參數(shù)的光強(qiáng)度分析。

52.Biosensor-Enabled Multiplexed On-Site Therapeutic Drug Monitoring of Antibiotics.

生物傳感器支持的抗生素多重現(xiàn)場(chǎng)治療藥物監(jiān)測(cè)。

53.Silk Embolic Material for Catheter-Directed Endovascular Drug Delivery.

用于導(dǎo)管引導(dǎo)血管內(nèi)藥物輸送的絲栓塞材料。

54.Extreme Environmental Thermal Shock Induced Dislocation-Rich Pt Nanoparticles Boosting Hydrogen Evolution Reaction.

極端環(huán)境熱沖擊引起的富含位錯(cuò)的 Pt 納米顆粒促進(jìn)析氫反應(yīng)。

55.Extracellular Matrix in Synthetic Hydrogel-Based Prostate Cancer Organoids Regulate Therapeutic Response to EZH2 and DRD2 Inhibitors.

基于合成水凝膠的前列腺癌類器官中的細(xì)胞外基質(zhì)調(diào)節(jié)對(duì) EZH2 和 DRD2 抑制劑的治療反應(yīng)。

56.Design of Quasi-MOF Nanospheres as a Dynamic Electrocatalyst toward Accelerated Sulfur Reduction Reaction for High-Performance Lithium–Sulfur Batteries.

準(zhǔn) MOF 納米球作為動(dòng)態(tài)電催化劑的設(shè)計(jì)，用于加速高性能鋰硫電池的硫還原反應(yīng)。

57.Polarimetric Image Sensor and Fermi Level Shifting Induced Multichannel Transition Based on 2D PdPS.

基于 2D PdPS 的偏振圖像傳感器和費(fèi)米能級(jí)移動(dòng)引起的多通道躍遷。

58.Atomically Dispersed Zinc(I) Active Sites to Accelerate Nitrogen Reduction Kinetics for Ammonia Electrosynthesis.

原子分散的鋅 (I) 活性位點(diǎn)加速氨電合成的氮還原動(dòng)力學(xué)。

59.Anti-Counterfeiting White Light Printed Image Multiplexing by Fast Nanosecond Laser Processing.

通過快速納秒激光處理實(shí)現(xiàn)防偽白光印刷圖像復(fù)用。

60.A Schottky-Barrier-Free Plasmonic Semiconductor Photocatalyst for Nitrogen Fixation in a “One-Stone-Two-Birds” Manner.

一種用于“一石二鳥”固氮的肖特基無勢(shì)壘等離子體半導(dǎo)體光催化劑。

61.Ultrafast-Response/Recovery Flexible Piezoresistive Sensors with DNA-Like Double Helix Yarns for Epidermal Pulse Monitoring.

具有類 DNA 雙螺旋紗線的超快響應(yīng)/恢復(fù)柔性壓阻傳感器，用于表皮脈沖監(jiān)測(cè)。

62.Versatile Preparation of Mesoporous Single-Layered Transition-Metal Sulfide/Carbon Composites for Enhanced Sodium Storage.

用于增強(qiáng)鈉儲(chǔ)存的介孔單層過渡金屬硫化物/碳復(fù)合材料的多功能制備。

63.Asymmetric Elimination Reaction on Chiral Metal Surfaces.

手性金屬表面上的不對(duì)稱消除反應(yīng)。

64.Interpolation between W Dopant and Co Vacancy in CoOOH for Enhanced Oxygen Evolution Catalysis.

CoOOH 中 W 摻雜劑和 Co 空位之間的插值，用于增強(qiáng)析氧催化。

65.Magnetic and Optical Field Multi-Assisted Li–O2 Batteries with Ultrahigh Energy Efficiency and Cycle Stability.

具有超高能量效率和循環(huán)穩(wěn)定性的磁光場(chǎng)多輔助Li-O2電池。

66.Ultrathin 2D NbWO6 Perovskite Semiconductor Based Gas Sensors with Ultrahigh Selectivity under Low Working Temperature.

基于超薄二維 NbWO6 鈣鈦礦半導(dǎo)體的氣體傳感器，在低工作溫度下具有超高選擇性。

67.3D Printed MXene Aerogels with Truly 3D Macrostructure and Highly Engineered Microstructure for Enhanced Electrical and Electrochemical Performance.

3D 打印 MXene 氣凝膠具有真正的 3D 宏觀結(jié)構(gòu)和高度工程化的微觀結(jié)構(gòu)，可增強(qiáng)電氣和電化學(xué)性能。